Entwicklung eines physikalischen Modells zur Beschreibung polarisationsaufgelöster, stoßinduzierter Energietransferprozesse kleiner Radikale in Flammen: ps-LIF Messungen und Simulationen von OH und NO (English shop)

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Within the scope of this work, not only were the most detailed polarization-resolved measurements on the OH radical to date presented, but above all a unified, sustainable model was developed with which all aspects of polarization-resolved fluorescence in atmospheric flames can be simulated in agreement with measurement results. In addition, NO measurements were carried out. Here, following A-X excitation into the vibrational levels v’ = 0 and v’ = 2, the rotational structure and the quenching behaviour were investigated. Both have hitherto either not been described at all or only incompletely in the literature.